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翻訳と辞書　辞書検索 [ 開発暫定版 ] スポンサード リンク Pressure-induced hydration ： ウィキペディア英語版 Pressure-induced hydration Pressure-induced hydration (PIH), also known as “super-hydration”, is a special case of pressure-induced insertion whereby water molecules are injected into the pores of microporous materials. In PIH, a microporous material is placed under pressure in the presence of water in the pressure-transmitting fluid of a diamond anvil cell.〔http://www.scientificamerican.com/article/crystals-strange-behavior/〕〔http://www.nature.com/nmat/journal/v2/n1/full/nmat805.html〕 Early physical characterization〔Moroz et al., Microporous and Mesoporous Materials 42 113 (2001)〕 and initial diffraction experiments〔R. M. Hazen, Science, 219, 1065 (1983)〕 in zeolites were followed by the first unequivocal structural characterization of PIH in the small-pore zeolite natrolite (Na16Al16Si24O80 x 16H2O), which in its fully super-hydrated form, Na16Al16Si24O80 x 32H2O, doubles〔Y. Lee, J.A. Hriljac, T. Vogt, J. B. Parise, G. Artioli, J. Am. Chem. Soc. 2001, 123, 12732-12733〕 the amount of water it contains in its pores. PIH has now been demonstrated in natrolites containing Li, K, Rb and Ag as monovalent cations〔D. Seoung, Y. Lee, CC Kao, T. Vogt, Y. Lee, Chem. Eur. J. 2013, 19, 10876-10883〕〔Y. Lee, D. Seoung, Y-N Jang, T. Vogt, Y. Lee, Chem. Eur. J. 2013, 19, 5806-5811〕 as well as in large-pore zeolites,〔M. Colligan, P.M. Forster, A.K. Cheetham, Y. Lee, T. Vogt, J.A. Hriljac J. Am. Chem. Soc. 2004, 126, 12015-12022〕 pyrochlores,〔P.W. Barnes, P.M. Woodward, Y. Lee, T. Vogt, J.A. Hriljac J. Am. Chem. Soc., 2003, 125 (15), pp 4572–4579〕 clays〔Shujie You, Daniel Kunz, Matthias Stöter, Hussein Kalo, Bernd Putz, Josef Breu, Alexandr V. Talyzin. Angewandte Chemie International Edition, 2013; 52 (14): 3891〕 and graphite oxide.〔Alexandr V. Talyzin, Vladimir L. Solozhenko, Oleksandr O. Kurakevych, Tams Szab, Imre Dekany, Alexandr Kurnosov, and Vladimir Dmitriev Angew. Chem. Int. Ed. 2008, 47, 8268 –8271〕 Using the noble gases Ar, Kr, and Xe as well as CO2 as pressure-transmitting fluids, researchers have prepared and structurally characterized the products of reversible, pressure-induced insertion of Ar〔Y. Lee, J.A. Hriljac, T. Vogt J. Phys. Chem. C 114, 6922-6927 (2010)〕 Kr,〔Donghoon Seoung, Yongmoon Lee, Hyunchae Cynn, Changyong Park, Kwang-Yong Choi, Douglas A Blom, William J Evans, Chi-Chang Kao, Thomas Vogt, Yongjae Lee, Nature chemistry 6(9), 835-829 (2014)〕 and CO2〔Y. Lee, D. Liu, D. Seoung, Z. Liu, CC Kao, T. Vogt J. Am. Chem. Soc. 2011, 133(6), 1674 - 1677〕 as well as the irreversible insertion of Xe〔 and water.〔Yongjae Lee, Thomas Vogt, Joseph A. Hriljac, John B. Parise, Jonathan C. Hanson & Sun Jin Kim, Nature 420, 485-489 (2002)〕 ==References== 抄文引用元・出典: フリー百科事典『 ウィキペディア（Wikipedia）』 ■ウィキペディアで「Pressure-induced hydration」の詳細全文を読む スポンサード リンク 翻訳と辞書 : 翻訳のためのインターネットリソース Copyright(C) kotoba.ne.jp 1997-2016. All Rights Reserved.